『Abstract
Urban soils act as the repository for a number of environmental
burdens, including Pb. Significant attention has been devoted
to reducing Pb burdens to children with outstanding success, but
the fact that blood Pb levels above 10μg/dL are disproportionately
found in children living in many USA cities (15-20% in some cities
compared to a national average of less than 2%) indicates that
not all of the sources have been eliminated. Although the health
risk of fine particulates has begun to raise concerns in cities,
little attention has been paid to Pb associated with these particulates
and the potential role of this pathway for continued Pb burdens
of urban youth. This review summarizes recent work on particulate
resuspension and the role of resuspension of Pb-enriched urban
soils as a continued source of bio-available Pb both outside and
inside homes, then presents recent efforts to model Pb burdens
to children based on the atmospheric parameters that drive particulate
resuspension. A strong seasonal relationship is found between
atmospheric particulate loading and blood Pb levels in children,
and new particulate loading models are presented for a range of
US cities involved in the Interagency Monitoring of Protected
Visual Environments (IMPROVE) program. These seasonal particulate
loading models have implications for a number of respiratory health
impacts, but can also be used to calculate seasonal patterns in
bio-available Pb redistribution onto contact surfaces (the primary
pathway for ingestion-related uptake in toddlers) and assist clinicians
in interpreting time-specific blood Pb tests.』
Contents
1. Introduction
2. Review of soil Pb, particulate resuspension and blood lead
2.1. Urban soil Pb
2.2. Urban soil Pb topology
2.3. Roadside soil resuspension
2.4. Soil resuspension as a contributor to PM10
2.5. Reducation in household Pb loading due to soil abatement
2.6. Transport of Pb from outside to inside
2.6.1. Particulate penetration and air exchange rates
2.6.2. Exterior Pb loading and indoor Pb penetration
2.7. Source apportionment of Pb in house dust
2.8. Association between soil Pb and blood Pb study designs
2.8.1. Association between soil Pb and blood Pb study designs:
cross-sectional
2.8.2. Association between soil Pb and blood Pb study designs:
ecological-spatial
2.8.3. Association between soil Pb and blood Pb study designs:
ecological-temporal
2.8.4. Association between soil Pb and blood Pb study designs:
prospective soil removal
2.8.5. Association between soil Pb and blood Pb study designs:
Descriptive
2.8.6. Blood Pb seasonality
2.8.7. Blood Pb seasonality and climate forcing
2.8.8. Alternative theories of blood Pb seasonality
3. New directions in soil resuspension and Pb loading
3.1. Methods
3.1.1. Data
3.1.2. Statistical model
4. Results
4.1. Hypothesis #1 - USA atmospheric soil seasonality
4.2. Hypothesis #2- atmospheric soil prediction model
5. Discussion
6. Conclusions
Acknowledgements
References